Hi Álvaro,
I guess you have already looked at gr-qc/0607025, where the package Harmonics is briefly described in the last appendix. I'm afraid we didn't write more documentation than that and the Harmonics.nb notebook itself.
I just tried to Get the package with the last version of xAct and there are no errors, so I think the package is still functional. I also evaluated the definition notebook and I indeed got some harmless-looking errors, like the fact that a function Laplacian is defined, but now there is a Laplacian symbol in Wolfram Language. This requires a renaming. Thanks for pointing this out.
Cheers,
Jose.