What type of flow is your model under-estimating? If stormflow, then increase CNs. If baseflow, then decrease CNs and reduce AWC. To reduce ET and increase water yield (flow), you need to minimize soil moisture by either reducing infiltration (higher CNs and stormflow) or passing the water more quickly through the soil layer (lower AWC). I'd also maximize ESCO also and reduce REVAP. Finally you could modify the plant cover parameters (like reducing LAI, CANMAX? etc.), but I know less about those manipulations.
-- Jim