Sounds like you are on the right track. Just keep in mind, while you may have had one address for your CIFS server on the Celerra, you will want a pool of addresses (at least one per node per subnet) on the Isilon with the name being an NS record pointing to the service IP rather than an A record that points to one node. The idea behind SmartConnect (even basic without the license) is to try and balance the clients across all the nodes without the clients needing any special software or have any knowledge of the Isilon. It's a pretty slick idea once you get it.
If your clients are SMB, there is no reason for addresses to move in the case of a failure and they won't in a static pool. The reason is that SMB clients do not follow an IP address if it moves. Even with SMB3 with CA, the client negotiates multiple addresses and moves to a new address upon failure. An SMB2 client will drop the connection and then next time a user tries to access the share, it will get a new address via SmartConnect (because we return a TTL of 0) and then it reconnects to a live node. For addresses to move upon a node failure, which is used by NFS clients, you would have a dynamic pool for your SmartConnect zone. But dynamic pools require the advanced license and if you don't have it, that option will be greyed out in the WebUI and not allowed on the CLI or with the API. But if you do not have NFS clients, dynamic zones aren't necessary since SMB behaves differently anyway.
My thought would be to have an NS record for each CIFS server you had on your Celerras. Each CIFS server name would be either the name of a SmartConnect zone or an alias to an SC zone if they are to share the same IP pool. That way each of your old CIFS server will have access to all of your nodes. This is good for redundancy as well as performance. NIC failover with your two 10Gb ports is fine and with tagging the aggr interface can live on all of your subnets.
Understanding IP pools and SmartConnect is an important part of setting up an Isilon, IMHO. If you need help with that, I'd start by reaching out to your Isilon SE. Those folks should know this stuff cold.