Sounds like a calculation mistake! Two things come to my mind:
1) Due to misspecification (or misprojection) of the coordinate reference system, calculations are blown up
2) More likely that you have a simpler calculation mistake around the lines of
output_variables = {
'TotalPM25':'PrimaryPM25 + pNH4 + pSO4 + pNO3 + SOA',
'deathsK':'(exp(log(1.06)/10 * TotalPM25) - 1) * TotalPop * 1.0465819687408728 * MortalityRate / 100000 * 1.025229357798165',
'deathsL':'(exp(log(1.14)/10 * TotalPM25) - 1) * TotalPop * 1.0465819687408728 * MortalityRate / 100000 * 1.025229357798165',
}"
As these lines include taking exponential, logarithm, and multiplication and also there is a division in the end, if you messed up in these lines it might cause such a big number.
Good luck!
Anil