Hi Kyle,
If I understand correctly, you want to remove dt(u)/Pr and -u dot grad(u)/Pr from your momentum equation? That's the right thing to do to work in the infinite Pr limit, but you will need to make some additional changes–I think that once you remove those terms, you will now be trying to solve for more dependent variables than necessary, and a 'Factor is exactly singular error' will occur.
I think what I would recommend is trying to eliminate the pressure variable from the problem and replacing u by a scalar streamfunction. I believe that if you take the curl of your new momentum equation you would end up with a biharmonic equation for the streamfunction involving T. You will have the same number of boundary conditions as before (rewriting the four for u in terms of the streamfunction), but there is no need for p nor its gauge constraint. I think you should end up solving for: a streamfunction, T, and six scalar tau fields.
There are probably other valid ways of going about this, but the key insight is that your Dedalus error is due to attempting to solve for the same number of dependent variables after dropping the inertial terms. I hope this advice helps!
Best,
Ben