Hi Rick
There are standard dimensions for Braille, and experienced readers of Braille can get pretty annoyed if the dimensions are wrong. I'm not sure, however, if it's considered acceptable to make the braille larger for children who are just learning to read it. Maybe Lore can weigh-in on that.
The print letter on the tile should probably be larger than this, through. Even so, you might find that each tile is so small that the prints will be distorted because each layer doesn't cool sufficiently before moving on to the next layer. You can slow down to allow more cooling time, but the plastic won't cool very well with the not nozzle staying that close to it. The solution to this problem is to print several tiles at the same time. This forces the nozzle to move away from each part (to work on the other ones), which gives them time to cool. A TAM is a pretty big machine, so I imagine it wouldn't be difficult to print the entire alphabet at once. You may, however, want to arrange the pieces so that the letters are all facing outward (toward the edges of the platform) with no other pieces in front of them. This ensures that if there are any print artifacts caused by retracting and moving between parts (which can be rough and uncomfortable to touch), they will be on the back faces of the tiles.