Scott,
I've used the Neo-Retro as a front brake for about ten years and have always had great luck with it. It looks great and, at the time, I was under the impression that the Neo-Retro was the more powerful brake—than the Touring Canti, that is. Paul's web page for the Neo-Retro used to warn that it's a powerful enough brake that one should make sure the frame could take the braking force, and maybe use the Touring Canti instead if one wasn't sure. I can no longer find that warning on the website. In any case, the Neo-Retro is powerful enough for me and relatively easy to adjust, and it's my first choice for a rim brake. (For some reason, likely user error/dimwittedness, I've never had luck with linear-pull brakes, but then I've never tried the Motolite.)
I chose the Touring Canti for the rear to maximize heel and pannier clearance. The combination works well for me, even with a full touring load going downhill.
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Bob