We develop a conceptual model that describes the transitions in the operationalization of solar radiation modification (SRM) as a climate intervention to reduce impacts from anthropogenic greenhouse gas forcing of the climate system. We distinguish predevelopment, postdevelopment, and postdeployment phases of SRM operationalization. We explore the interactions between the human system and climate system that drive transitions between these stages in the emergence of SRM as a climate intervention. We discuss the insights around SRM development and deployment that emerge from this conceptual model.